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  • Chain Walking of Allylrhodium Species Towards Esters During Rhodium‐Catalysed Nucleophilic Allylations of Imines

    • Chain Walking of Allylrhodium Species Towards Esters During Rhodium‐Catalysed Nucleophilic Allylations of Imines

    Title Chain Walking of Allylrhodium Species Towards Esters During Rhodium‐Catalysed Nucleophilic Allylations of Imines
    Authors Dr. Jose I. Martínez, Joshua J. Smith, Dr. Hamish B. Hepburn, Prof. Hon Wai Lam
    Magazine Angewandte Chemie (International Ed. in English)
    Date 12/03/2015
    DOI 10.1002/anie.201508964
    Introduction Allylrhodium species formed from δ‐trifluoroboryl β,γ‐unsaturated esters can migrate towards ester groups. These allylrhodium species then react with imines, producing compounds with two new stereocentres and a Z‐alkene. Utilising a chiral diene ligand allows for products with high enantioselectivities, manifesting a significant matched/mismatched effect with the allyltrifluoroborate's chirality.
    Quote José I. Martínez-Guerrero, Joshua J. Smith and Hamish B Hepburn et al. Chain Walking of Allylrhodium Species Towards Esters During Rhodium‐Catalysed Nucleophilic Allylations of Imines. Angew. Chem. Int. Ed. Engl. 2015. DOI: 10.1002/anie.201508964
    Element Rhodium (Rh) , Boron (B)
    Industry Chemical & Pharmacy
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