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  • Enantioselective Rhodium‐Catalyzed Coupling of Arylboronic Acids, 1,3‐Enynes, and Imines by Alkenyl‐to‐Allyl 1,4‐Rhodium(I) Migration

    • Enantioselective Rhodium‐Catalyzed Coupling of Arylboronic Acids, 1,3‐Enynes, and Imines by Alkenyl‐to‐Allyl 1,4‐Rhodium(I) Migration

    Title Enantioselective Rhodium‐Catalyzed Coupling of Arylboronic Acids, 1,3‐Enynes, and Imines by Alkenyl‐to‐Allyl 1,4‐Rhodium(I) Migration
    Authors Michael Callingham, Dr. Benjamin M. Partridge, Dr. William Lewis, Prof. Hon Wai Lam
    Magazine Angewandte Chemie (International Ed. in English)
    Date 11/24/2017
    DOI 10.1002/anie.201709334
    Introduction A chiral rhodium complex acts as a catalyst for the highly enantioselective coupling of arylboronic acids, 1,3-enynes, and imines, resulting in the formation of homoallylic sulfamates. The crucial step in this process is the conversion of alkenyl-rhodium(I) to allylrhodium(I) species through 1,4-rhodium(I) migration.
    Quote Michael Callingham, Benjamin M. Partridge, William Lewis et al. Enantioselective Rhodium‐Catalysed Coupling of Arylboronic Acids, 1,3‐Enynes, and Imines by Alkenyl‐to‐Allyl 1,4‐Rhodium(I) Migration. Angew. Chem. Int. Ed. Engl. 2017. DOI: 10.1002/anie.201709334
    Element Rhodium (Rh)
    Materials Chemical Compounds
    Industry Chemical & Pharmacy
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