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  • Remote C−H Glycosylation by Ruthenium(II) Catalysis: Modular Assembly of meta‐ C‐Aryl Glycosides

    • Remote C−H Glycosylation by Ruthenium(II) Catalysis: Modular Assembly of meta‐ C‐Aryl Glycosides

    Title Remote C−H Glycosylation by Ruthenium(II) Catalysis: Modular Assembly of meta‐ C‐Aryl Glycosides
    Authors Jun Wu, Nikolaos Kaplaneris, Julia Pöhlmann, Takuya Michiyuki, Binbin Yuan, Lutz Ackermann
    Magazine Angewandte Chemie (International Ed. in English)
    Date 09/13/2022
    DOI 10.1002/anie.202208620
    Introduction C-aryl glycosides are essential in natural products and pharmaceuticals, influencing efficient synthesis methods. Traditional cross-coupling often utilises palladium catalysts with prefunctionalised substrates. This study presents a method using ruthenium(II)-catalysed meta-C−H glycosylation, allowing access to meta-C-aryl glycosides from readily available glycosyl halide donors. The process benefits from mild reaction conditions, exceptional anomeric selectivity, and exclusive meta-site selectivity, demonstrating the efficiency of ruthenium catalysis.
    Quote Jun Wu, Nikolaos Kaplaneris and Julia Pöhlmann et al. Remote C−H Glycosylation by Ruthenium(II) Catalysis: Modular Assembly of meta‐C‐Aryl Glycosides. Angew. Chem. Int. Ed. Engl. 2022. DOI: 10.1002/anie.202208620
    Element Ruthenium (Ru)
    Industry Chemical & Pharmacy
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